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Two-dimensional electron gas with universal subbands at the surface of SrTiO3

Abstract : As silicon is the basis of conventional electronics, so strontium titanate (SrTiO3) is the foundation of the emerging field of oxide electronics1,2.SrTiO3 is the preferred template for the creation of exotic, two-dimensional (2D) phases of electronmatter at oxide interfaces3-5 that have metal-insulator transitions6,7, superconductivity8,9 or large negative magnetoresistance10. However, the physical nature of the electronic structure underlying these 2D electron gases (2DEGs), which is crucial to understanding their remarkable properties11,12, remains elusive. Here we show, using angle-resolved photoemission spectroscopy, that there is a highly metallic universal 2DEG at the vacuum-cleaved surface of SrTiO3 (including the non-doped insulating material) independently of bulk carrier densities over more than seven decades. This 2DEG is confined within a region of about five unit cells and has a sheet carrier density of 0.33 electrons per square lattice parameter. The electronic structure consists of multiple subbands of heavy and light electrons. The similarity of this 2DEG to those reported in SrTiO3-based heterostructures6,8,13 and field-effect transistors9,14 suggests that different forms of electron confinement at the surface of SrTiO3 lead to essentially the same 2DEG. Our discovery provides a model system for the study of the electronic structure of 2DEGs in SrTiO3-based devices and a novel means of generating 2DEGs at the surfaces of transition-metal oxides.
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http://hal.in2p3.fr/in2p3-00558473
Contributor : Christine Hadrossek <>
Submitted on : Friday, January 28, 2011 - 1:54:50 PM
Last modification on : Wednesday, September 16, 2020 - 5:42:34 PM

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A. F. Santander-Syro, O. Copie, T. Kondo, S. Fortuna, S. Pailhes, et al.. Two-dimensional electron gas with universal subbands at the surface of SrTiO3. Nature, Nature Publishing Group, 2011, 469, pp.189-194. ⟨10.1038/nature09720⟩. ⟨in2p3-00558473⟩

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