Velocity of a Molecule Evaporated from a Water Nanodroplet: Maxwell–Boltzmann Statistics versus Non-Ergodic Events

Abstract : The velocity distribution of water molecules evaporated from a mass-selected protonated water nanodroplet after a collision-induced electronic excitation is reported. In their Communication (DOI: 10.1002/anie.201505890), M. Farizon et al. show that besides the Maxwell–Boltzmann statistics behavior, a distinct high-velocity contribution provides evidence for molecular evaporation before complete energy redistribution, corresponding to non-ergodic events.
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Angewandte Chemie International Edition, Wiley-VCH Verlag, 2015, 54, pp.14685-14689. 〈http://onlinelibrary.wiley.com/doi/10.1002/anie.201505890/epdf〉. 〈10.1002/anie.201509527〉
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Soumis le : mardi 27 octobre 2015 - 10:35:40
Dernière modification le : jeudi 15 mars 2018 - 11:40:10

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H. Abdoul-Carime, F. Berthias, L. Feketeová, M. Marciante, F. Calvo, et al.. Velocity of a Molecule Evaporated from a Water Nanodroplet: Maxwell–Boltzmann Statistics versus Non-Ergodic Events. Angewandte Chemie International Edition, Wiley-VCH Verlag, 2015, 54, pp.14685-14689. 〈http://onlinelibrary.wiley.com/doi/10.1002/anie.201505890/epdf〉. 〈10.1002/anie.201509527〉. 〈in2p3-01220955〉

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